I've never gotten any clear answers on this. Most people seem to think that either they can't get a full 60 Rc (even though it says so there) or that they think bainite wouldn't hold an edge as long. There are some conflicting reports on wear resistance, it would be very interesting to see some rope cutting or CATRA comparing bainite vs. martensite at the same hardness. I learned the other day that the reason bainite is tougher is because it is a stable phase rather than unstable (i.e. martensite), also it doesn't have the same shock in quenching, of course. I don't have any salt pots; I've heard that salt pots can be hard to maintain, are a little dangerous, etc. I'm mostly interested in stainless steels, so bainite isn't something I've ever had a major interest in, but 52100 is just about the best steel to try it with.
Edit: It wouldn't hurt to go in to cryo after and then temper, though it may or may not be necessary.